%0 Journal Article %1 AENM:AENM201701659 %A Yu, Zhenhua %A Zhang, Linxing %A Tian, Sen %A Zhang, Fan %A Zhang, Bin %A Niu, Fangfang %A Zeng, Pengju %A Qu, Junle %A Rudd, Peter Neil %A Huang, Jinsong %A Lian, Jiarong %D 2017 %J Advanced Energy Materials %K optimization perovskite transport %P n/a--n/a %R 10.1002/aenm.201701659 %T Hot-Substrate Deposition of Hole- and Electron-Transport Layers for Enhanced Performance in Perovskite Solar Cells %U http://dx.doi.org/10.1002/aenm.201701659 %X Charge transport layers play an important role in determining the power conversion efficiencies (PCEs) of perovskite solar cells (PSCs). However, it has proven challenging to produce thin and compact charge transport layers via solution processing techniques. Herein, a hot substrate deposition method capable of improving the morphology of high-coverage hole-transport layers (HTLs) and electron-transport layers (ETLs) is reported. PSC devices using HTLs deposited on a hot substrate show improvement in the open-circuit voltage (Voc) from 1.041 to 1.070 V and the PCE from 17.00% to 18.01%. The overall device performance is then further enhanced with the hot substrate deposition of ETLs as the Voc and PCE reach 1.105 V and 19.16%, respectively. The improved performance can be explained by the decreased current leakage and series resistance, which are present in PSCs with rough and discontinuous HTLs and ETLs.

@article{AENM:AENM201701659, abstract = {Charge transport layers play an important role in determining the power conversion efficiencies (PCEs) of perovskite solar cells (PSCs). However, it has proven challenging to produce thin and compact charge transport layers via solution processing techniques. Herein, a hot substrate deposition method capable of improving the morphology of high-coverage hole-transport layers (HTLs) and electron-transport layers (ETLs) is reported. PSC devices using HTLs deposited on a hot substrate show improvement in the open-circuit voltage (Voc) from 1.041 to 1.070 V and the PCE from 17.00% to 18.01%. The overall device performance is then further enhanced with the hot substrate deposition of ETLs as the Voc and PCE reach 1.105 V and 19.16%, respectively. The improved performance can be explained by the decreased current leakage and series resistance, which are present in PSCs with rough and discontinuous HTLs and ETLs.}, added-at = {2017-11-14T11:21:20.000+0100}, author = {Yu, Zhenhua and Zhang, Linxing and Tian, Sen and Zhang, Fan and Zhang, Bin and Niu, Fangfang and Zeng, Pengju and Qu, Junle and Rudd, Peter Neil and Huang, Jinsong and Lian, Jiarong}, biburl = {https://www.bibsonomy.org/bibtex/22d566d7e0862e63fc30c91a375f4a097/bretschneider_m}, doi = {10.1002/aenm.201701659}, interhash = {c44d23857b327bf8bb7a7d022ee50667}, intrahash = {2d566d7e0862e63fc30c91a375f4a097}, issn = {1614-6840}, journal = {Advanced Energy Materials}, keywords = {optimization perovskite transport}, pages = {n/a--n/a}, timestamp = {2017-11-14T11:23:30.000+0100}, title = {Hot-Substrate Deposition of Hole- and Electron-Transport Layers for Enhanced Performance in Perovskite Solar Cells}, url = {http://dx.doi.org/10.1002/aenm.201701659}, year = 2017 }