%0 Journal Article %1 ADMA:ADMA201703256 %A Hu, Wei %A Huang, Wei %A Yang, Shuzhen %A Wang, Xiao %A Jiang, Zhenyu %A Zhu, Xiaoli %A Zhou, Hong %A Liu, Hongjun %A Zhang, Qinglin %A Zhuang, Xiujuan %A Yang, Junliang %A Kim, Dong Ha %A Pan, Anlian %D 2017 %J Advanced Materials %K high perovskite photodetector quality %P n/a--n/a %R 10.1002/adma.201703256 %T High-Performance Flexible Photodetectors based on High-Quality Perovskite Thin Films by a Vapor–Solution Method %U http://dx.doi.org/10.1002/adma.201703256 %X Organometal halide perovskites are new light-harvesting materials for lightweight and flexible optoelectronic devices due to their excellent optoelectronic properties and low-temperature process capability. However, the preparation of high-quality perovskite films on flexible substrates has still been a great challenge to date. Here, a novel vapor–solution method is developed to achieve uniform and pinhole-free organometal halide perovskite films on flexible indium tin oxide/poly(ethylene terephthalate) substrates. Based on the as-prepared high-quality perovskite thin films, high-performance flexible photodetectors (PDs) are constructed, which display a nR value of 81 A W−1 at a low working voltage of 1 V, three orders higher than that of previously reported flexible perovskite thin-film PDs. In addition, these flexible PDs exhibit excellent flexural stability and durability under various bending situations with their optoelectronic performance well retained. This breakthrough on the growth of high-quality perovskite thin films opens up a new avenue to develop high-performance flexible optoelectronic devices.

@article{ADMA:ADMA201703256, abstract = {Organometal halide perovskites are new light-harvesting materials for lightweight and flexible optoelectronic devices due to their excellent optoelectronic properties and low-temperature process capability. However, the preparation of high-quality perovskite films on flexible substrates has still been a great challenge to date. Here, a novel vapor–solution method is developed to achieve uniform and pinhole-free organometal halide perovskite films on flexible indium tin oxide/poly(ethylene terephthalate) substrates. Based on the as-prepared high-quality perovskite thin films, high-performance flexible photodetectors (PDs) are constructed, which display a nR value of 81 A W−1 at a low working voltage of 1 V, three orders higher than that of previously reported flexible perovskite thin-film PDs. In addition, these flexible PDs exhibit excellent flexural stability and durability under various bending situations with their optoelectronic performance well retained. This breakthrough on the growth of high-quality perovskite thin films opens up a new avenue to develop high-performance flexible optoelectronic devices.}, added-at = {2017-10-16T10:59:27.000+0200}, author = {Hu, Wei and Huang, Wei and Yang, Shuzhen and Wang, Xiao and Jiang, Zhenyu and Zhu, Xiaoli and Zhou, Hong and Liu, Hongjun and Zhang, Qinglin and Zhuang, Xiujuan and Yang, Junliang and Kim, Dong Ha and Pan, Anlian}, biburl = {https://www.bibsonomy.org/bibtex/24474aa5381c86c9ea2f1ff690ecaca9d/fabianopkm}, description = {High-Performance Flexible Photodetectors based on High-Quality Perovskite Thin Films by a Vapor–Solution Method - Hu - 2017 - Advanced Materials - Wiley Online Library}, doi = {10.1002/adma.201703256}, interhash = {23bba3124f9533edb64e28826c8f2356}, intrahash = {4474aa5381c86c9ea2f1ff690ecaca9d}, issn = {1521-4095}, journal = {Advanced Materials}, keywords = {high perovskite photodetector quality}, pages = {n/a--n/a}, timestamp = {2017-10-16T10:59:27.000+0200}, title = {High-Performance Flexible Photodetectors based on High-Quality Perovskite Thin Films by a Vapor–Solution Method}, url = {http://dx.doi.org/10.1002/adma.201703256}, year = 2017 }