%0 Journal Article %1 PhysRevLett.126.176403 %A Vidal, R. C. %A Bentmann, H. %A Facio, J. I. %A Heider, T. %A Kagerer, P. %A Fornari, C. I. %A Peixoto, T. R. F. %A Figgemeier, T. %A Jung, S. %A Cacho, C. %A Büchner, B. %A van den Brink, J. %A Schneider, C. M. %A Plucinski, L. %A Schwier, E. F. %A Shimada, K. %A Richter, M. %A Isaeva, A. %A Reinert, F. %D 2021 %I American Physical Society %J Phys. Rev. Lett. %K b %N 17 %P 176403 %R 10.1103/PhysRevLett.126.176403 %T Orbital complexity in intrinsic magnetic topological insulators MnBi$_4$Te$_7$ and MnBi$_6$Te$_10$ %U https://link.aps.org/doi/10.1103/PhysRevLett.126.176403 %V 126 %X Using angle-resolved photoelectron spectroscopy (ARPES), we investigate the surface electronic structure of the magnetic van der Waals compounds MnBi4Te7 and MnBi6Te10, the n=1 and 2 members of a modular ($Bi_2Te_3$)n($MnBi_2Te_4$) series, which have attracted recent interest as intrinsic magnetic topological insulators. Combining circular dichroic, spin-resolved and photon-energy-dependent ARPES measurements with calculations based on density functional theory, we unveil complex momentum-dependent orbital and spin textures in the surface electronic structure and disentangle topological from trivial surface bands. We find that the Dirac-cone dispersion of the topologial surface state is strongly perturbed by hybridization with valence-band states for $Bi_2Te_3$-terminated surfaces but remains preserved for MnBi2Te4-terminated surfaces. Our results firmly establish the topologically nontrivial nature of these magnetic van der Waals materials and indicate that the possibility of realizing a quantized anomalous Hall conductivity depends on surface termination.

@article{PhysRevLett.126.176403, abstract = {Using angle-resolved photoelectron spectroscopy (ARPES), we investigate the surface electronic structure of the magnetic van der Waals compounds MnBi4Te7 and MnBi6Te10, the n=1 and 2 members of a modular ($Bi_2Te_3$)n($MnBi_2Te_4$) series, which have attracted recent interest as intrinsic magnetic topological insulators. Combining circular dichroic, spin-resolved and photon-energy-dependent ARPES measurements with calculations based on density functional theory, we unveil complex momentum-dependent orbital and spin textures in the surface electronic structure and disentangle topological from trivial surface bands. We find that the Dirac-cone dispersion of the topologial surface state is strongly perturbed by hybridization with valence-band states for $Bi_2Te_3$-terminated surfaces but remains preserved for MnBi2Te4-terminated surfaces. Our results firmly establish the topologically nontrivial nature of these magnetic van der Waals materials and indicate that the possibility of realizing a quantized anomalous Hall conductivity depends on surface termination.}, added-at = {2021-05-27T10:17:21.000+0200}, author = {Vidal, R. C. and Bentmann, H. and Facio, J. I. and Heider, T. and Kagerer, P. and Fornari, C. I. and Peixoto, T. R. F. and Figgemeier, T. and Jung, S. and Cacho, C. and Büchner, B. and van den Brink, J. and Schneider, C. M. and Plucinski, L. and Schwier, E. F. and Shimada, K. and Richter, M. and Isaeva, A. and Reinert, F.}, biburl = {https://www.bibsonomy.org/bibtex/21e5c695e7e7942a92548b92c9e7e653f/ctqmat}, day = 28, description = {Phys. Rev. Lett. 126, 176403 (2021) - Orbital Complexity in Intrinsic Magnetic Topological Insulators ${\mathrm{MnBi}}_{4}{\mathrm{Te}}_{7}$ and ${\mathrm{MnBi}}_{6}{\mathrm{Te}}_{10}$}, doi = {10.1103/PhysRevLett.126.176403}, interhash = {2a7dc4ffccdd49acd99848336e8b95e4}, intrahash = {1e5c695e7e7942a92548b92c9e7e653f}, journal = {Phys. Rev. Lett.}, keywords = {b}, month = {04}, number = 17, numpages = {7}, pages = 176403, publisher = {American Physical Society}, timestamp = {2023-10-19T10:15:12.000+0200}, title = {Orbital complexity in intrinsic magnetic topological insulators MnBi$_{\mathbf{4}}$Te$_{\mathbf{7}}$ and MnBi$_{\mathbf{6}}$Te$_{\mathbf{10}}$}, url = {https://link.aps.org/doi/10.1103/PhysRevLett.126.176403}, volume = 126, year = 2021 }