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Magnetocaloric effect and spin-strain coupling in the spin-nematic state of LiCuVO$_4$

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Phys. Rev. Res., 1 (3): 033065 (31.10.2019)
DOI: 10.1103/PhysRevResearch.1.033065

Аннотация

We report on the magnetocaloric effect and ultrasound studies of the frustrated quasi-one-dimensional spin-1/2 compound $LiCuVO_4$, evidencing a spin-nematic state. The magnetic Grüneisen parameter diverges at the transition to the spin-nematic phase, μ0Hc3≈40 T, showing quantum criticality accompanied by entropy accumulation. The observed high-field anomalies in the acoustic properties clearly evidence a strong involvement of the lattice in the spin dynamics. The theoretical approach, based on exchange-striction coupling with dipolar and quadrupolar contributions, suggests that the spin-dipole-strain and quadrupole-strain interactions govern the spin-nematicity in $LiCuVO_4$.

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