Light absorption by aerosols is one of the most uncertain parameters associated with the direct and indirect aerosol effects on climate and is one of the most difficult quantities to measure. This article describes the development of a sensitive method of measuring aerosol absorption at 532 nm with excellent time response (detection limit: 0.08 Mm(-1), 60 second average) using photoacoustic absorption spectroscopy. An accurate calibration method (accuracy of 1-2%) at atmospherically relevant absorption levels and independent validation of the photoacoustic technique is presented. An upper limit to the instrument precision for aerosol absorption measurement is approximate to 6% (2 sigma, 30 sec) while instrument accuracy is calculated to be approximate to 5%. A standard for aerosol absorption measurement techniques using well characterized absorbing aerosol is also proposed.
Lack, Da
NOAA, Earth System Res Lab, 325 Broadway, Boulder, CO 80305 USA
NOAA, Earth System Res Lab, 325 Broadway, Boulder, CO 80305 USA
NOAA, Earth System Res Lab, Boulder, CO 80305 USA
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO USA
%0 Journal Article
%1 Lack:2006p330
%A Lack, D
%A Lovejoy, E
%A Baynard, T
%A Pettersson, A
%A Ravishankara, A. R
%D 2006
%J Aerosol Science and Technology
%K imported
%N 9
%P 697--708
%R Doi 10.1080/02786820600803917
%T Aerosol absorption measurement using photoacoustic spectroscopy: Sensitivity, calibration, and uncertainty developments
%U http://links.isiglobalnet2.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=mekentosj&SrcApp=Papers&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000238418800006
%V 40
%X Light absorption by aerosols is one of the most uncertain parameters associated with the direct and indirect aerosol effects on climate and is one of the most difficult quantities to measure. This article describes the development of a sensitive method of measuring aerosol absorption at 532 nm with excellent time response (detection limit: 0.08 Mm(-1), 60 second average) using photoacoustic absorption spectroscopy. An accurate calibration method (accuracy of 1-2%) at atmospherically relevant absorption levels and independent validation of the photoacoustic technique is presented. An upper limit to the instrument precision for aerosol absorption measurement is approximate to 6% (2 sigma, 30 sec) while instrument accuracy is calculated to be approximate to 5%. A standard for aerosol absorption measurement techniques using well characterized absorbing aerosol is also proposed.
@article{Lack:2006p330,
abstract = {Light absorption by aerosols is one of the most uncertain parameters associated with the direct and indirect aerosol effects on climate and is one of the most difficult quantities to measure. This article describes the development of a sensitive method of measuring aerosol absorption at 532 nm with excellent time response (detection limit: 0.08 Mm(-1), 60 second average) using photoacoustic absorption spectroscopy. An accurate calibration method (accuracy of 1-2%) at atmospherically relevant absorption levels and independent validation of the photoacoustic technique is presented. An upper limit to the instrument precision for aerosol absorption measurement is approximate to 6% (2 sigma, 30 sec) while instrument accuracy is calculated to be approximate to 5%. A standard for aerosol absorption measurement techniques using well characterized absorbing aerosol is also proposed.},
added-at = {2010-06-22T19:38:37.000+0200},
affiliation = {Lack, Da
NOAA, Earth System Res Lab, 325 Broadway, Boulder, CO 80305 USA
NOAA, Earth System Res Lab, 325 Broadway, Boulder, CO 80305 USA
NOAA, Earth System Res Lab, Boulder, CO 80305 USA
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO USA},
author = {Lack, D and Lovejoy, E and Baynard, T and Pettersson, A and Ravishankara, A. R},
biburl = {https://www.bibsonomy.org/bibtex/28b340de6b8486c8754186d3c69fec51f/gsmith},
date-added = {2010-03-10 16:47:33 -0500},
date-modified = {2010-04-29 13:23:09 -0400},
doi = {Doi 10.1080/02786820600803917},
interhash = {c5d909c781f730466751db09e459c6fe},
intrahash = {8b340de6b8486c8754186d3c69fec51f},
journal = {Aerosol Science and Technology},
keywords = {imported},
label = {rec-number 2062},
local-url = {file://localhost/Users/geoffreysmith/Documents/Papers/Aerosol%20Science%20and%20Technology/2006/Aerosol%20Science%20and%20Technology,%2040,%20697-708%202006.pdf},
month = Sep,
note = {054ZS
Times Cited:22
Cited References Count:39},
number = 9,
pages = {697--708},
pmid = {000238418800006},
rating = {0},
timestamp = {2010-06-22T19:39:29.000+0200},
title = {Aerosol absorption measurement using photoacoustic spectroscopy: Sensitivity, calibration, and uncertainty developments},
uri = {papers://E88B624E-D406-46FF-9D95-BB9C1AAE3FDC/Paper/p330},
url = {http://links.isiglobalnet2.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=mekentosj&SrcApp=Papers&DestLinkType=FullRecord&DestApp=WOS&KeyUT=000238418800006},
volume = 40,
year = 2006
}