We investigate the slow dynamics of a colloidal model with two repulsive
length scales, whose interaction potential is the sum of a hard-core and a
square shoulder. Despite the simplicity of the interactions, Mode-Coupling
theory predicts a complex dynamic scenario: a fluid-glass line with two
reentrances and a glass-glass line ending with multiple higher-order (\$A\_3\$ or
\$A\_4\$) singularities. In this work we verify the existence of the two \$A\_4\$
points by numerical simulations, observing subdiffusive behaviour of the
mean-square displacement and logarithmic decay of the density correlators.
Surprisingly, we also discover a novel dynamic behaviour generated by the
competition between the two higher-order singularities. This results in the
presence of special loci along which the dynamics is identical at all
length and time scales.
%0 Journal Article
%1 Gnan2014Multiple
%A Gnan, Nicoletta
%A Das, Gayatri
%A Sperl, Matthias
%A Sciortino, Francesco
%A Zaccarelli, Emanuela
%D 2014
%J Physical Review Letters
%K a-singularities, glass-glass-transition, mode-coupling-theory critical-phenomena glasses
%N 25
%R 10.1103/PhysRevLett.113.258302
%T Multiple Glass Singularities and Isodynamics in a Core-Softened Model for Glass-Forming Systems
%U http://dx.doi.org/10.1103/PhysRevLett.113.258302
%V 113
%X We investigate the slow dynamics of a colloidal model with two repulsive
length scales, whose interaction potential is the sum of a hard-core and a
square shoulder. Despite the simplicity of the interactions, Mode-Coupling
theory predicts a complex dynamic scenario: a fluid-glass line with two
reentrances and a glass-glass line ending with multiple higher-order (\$A\_3\$ or
\$A\_4\$) singularities. In this work we verify the existence of the two \$A\_4\$
points by numerical simulations, observing subdiffusive behaviour of the
mean-square displacement and logarithmic decay of the density correlators.
Surprisingly, we also discover a novel dynamic behaviour generated by the
competition between the two higher-order singularities. This results in the
presence of special loci along which the dynamics is identical at all
length and time scales.
@article{Gnan2014Multiple,
abstract = {We investigate the slow dynamics of a colloidal model with two repulsive
length scales, whose interaction potential is the sum of a hard-core and a
square shoulder. Despite the simplicity of the interactions, Mode-Coupling
theory predicts a complex dynamic scenario: a fluid-glass line with two
reentrances and a glass-glass line ending with multiple higher-order (\$A\_3\$ or
\$A\_4\$) singularities. In this work we verify the existence of the two \$A\_4\$
points by numerical simulations, observing subdiffusive behaviour of the
mean-square displacement and logarithmic decay of the density correlators.
Surprisingly, we also discover a novel dynamic behaviour generated by the
competition between the two higher-order singularities. This results in the
presence of special loci along which the dynamics is identical \textit{at all}
length and time scales.},
added-at = {2019-06-10T14:53:09.000+0200},
archiveprefix = {arXiv},
author = {Gnan, Nicoletta and Das, Gayatri and Sperl, Matthias and Sciortino, Francesco and Zaccarelli, Emanuela},
biburl = {https://www.bibsonomy.org/bibtex/20e87908e2f661084100b85381e7b2129/nonancourt},
citeulike-article-id = {13324390},
citeulike-linkout-0 = {http://dx.doi.org/10.1103/PhysRevLett.113.258302},
citeulike-linkout-1 = {http://arxiv.org/abs/1407.3917},
citeulike-linkout-2 = {http://arxiv.org/pdf/1407.3917},
day = 18,
doi = {10.1103/PhysRevLett.113.258302},
eprint = {1407.3917},
interhash = {5f8f83aa8765077c792b6783c898c2e1},
intrahash = {0e87908e2f661084100b85381e7b2129},
issn = {1079-7114},
journal = {Physical Review Letters},
keywords = {a-singularities, glass-glass-transition, mode-coupling-theory critical-phenomena glasses},
month = dec,
number = 25,
posted-at = {2014-08-13 10:58:32},
priority = {2},
timestamp = {2019-07-31T12:31:28.000+0200},
title = {{Multiple Glass Singularities and Isodynamics in a Core-Softened Model for Glass-Forming Systems}},
url = {http://dx.doi.org/10.1103/PhysRevLett.113.258302},
volume = 113,
year = 2014
}