The optical near-field in the vicinity of a metal tip is mapped using a single-molecule optical probe. We observe an enhancement of the fluorescence signal by a factor of 5.7±0.3, clearly larger than the fourfold enhancement that can arise from constructive interference if the tip acts as a simple mirror. Considering the tip apex as a nanoparticle of nonregular shape, we suggest that, in the case of gold tips, the enhancement is due to resonant plasmon excitation. Consistently, no enhancement has been observed using Pt/Ir tips.
Kramer et al. - 2002 - Optical near-field enhancement at a metal tip prob.pdf:C\:\\Users\\scherzad\\Zotero\\storage\\8WKDG4K6\\Kramer et al. - 2002 - Optical near-field enhancement at a metal tip prob.pdf:application/pdf;Snapshot:C\:\\Users\\scherzad\\Zotero\\storage\\25RS7PMN\\1.html:text/html
%0 Journal Article
%1 kramer2002optical
%A Kramer, Andrei
%A Trabesinger, Werner
%A Hecht, Bert
%A Wild, Urs P.
%D 2002
%J Appl. Phys. Lett.
%K experiment nano-optics near-field single-molecules
%N 9
%P 1652-1654
%R 10.1063/1.1453479
%T Optical near-field enhancement at a metal tip probed by a single fluorophore
%V 80
%X The optical near-field in the vicinity of a metal tip is mapped using a single-molecule optical probe. We observe an enhancement of the fluorescence signal by a factor of 5.7±0.3, clearly larger than the fourfold enhancement that can arise from constructive interference if the tip acts as a simple mirror. Considering the tip apex as a nanoparticle of nonregular shape, we suggest that, in the case of gold tips, the enhancement is due to resonant plasmon excitation. Consistently, no enhancement has been observed using Pt/Ir tips.
@article{kramer2002optical,
abstract = {The optical near-field in the vicinity of a metal tip is mapped using a single-molecule optical probe. We observe an enhancement of the fluorescence signal by a factor of 5.7±0.3, clearly larger than the fourfold enhancement that can arise from constructive interference if the tip acts as a simple mirror. Considering the tip apex as a nanoparticle of nonregular shape, we suggest that, in the case of gold tips, the enhancement is due to resonant plasmon excitation. Consistently, no enhancement has been observed using Pt/Ir tips.},
added-at = {2020-02-17T11:18:50.000+0100},
author = {Kramer, Andrei and Trabesinger, Werner and Hecht, Bert and Wild, Urs P.},
biburl = {https://www.bibsonomy.org/bibtex/22dfe148278b47850e29688e01341b976/ep5optics},
day = 25,
doi = {10.1063/1.1453479},
file = {Kramer et al. - 2002 - Optical near-field enhancement at a metal tip prob.pdf:C\:\\Users\\scherzad\\Zotero\\storage\\8WKDG4K6\\Kramer et al. - 2002 - Optical near-field enhancement at a metal tip prob.pdf:application/pdf;Snapshot:C\:\\Users\\scherzad\\Zotero\\storage\\25RS7PMN\\1.html:text/html},
interhash = {53bef3c5c91f2bd4670923d9638d66c6},
intrahash = {2dfe148278b47850e29688e01341b976},
issn = {0003-6951},
journal = {Appl. Phys. Lett.},
keywords = {experiment nano-optics near-field single-molecules},
month = {02},
number = 9,
pages = {1652-1654},
timestamp = {2020-02-17T11:18:50.000+0100},
title = {Optical near-field enhancement at a metal tip probed by a single fluorophore},
urldate = {2020-02-17},
volume = 80,
year = 2002
}