Graphene nano-optics at terahertz (THz) frequencies (ν) is theoretically anticipated to feature extraordinary effects. However, interrogating such phenomena is nontrivial, since the atomically thin graphene dimensionally mismatches the THz radiation wavelength reaching hundreds of micrometers. Greater challenges happen in the THz gap (0.1–10 THz) wherein light sources are scarce. To surpass these barriers, we use a nanoscope illuminated by a highly brilliant and tunable free-electron laser to image the graphene nano-optical response from 1.5 to 6.0 THz. For ν < 2 THz, we observe a metal-like behavior of graphene, which screens optical fields akin to noble metals, since this excitation range approaches its charge relaxation frequency. At 3.8 THz, plasmonic resonances cause a field-enhancement effect (FEE) that improves the graphene imaging power. Moreover, we show that the metallic behavior and the FEE are tunable upon electrical doping, thus providing further control of these graphene nano-optical properties in the THz gap.
Beschreibung
Graphene Nano-Optics in the Terahertz Gap | Nano Letters
%0 Journal Article
%1 noauthororeditor
%A Feres, Flávio H.
%A Barcelos, Ingrid D.
%A Cadore, Alisson R.
%A Wehmeier, Lukas
%A Nörenberg, Tobias
%A Mayer, Rafael A.
%A Freitas, Raul O.
%A Eng, Lukas M.
%A Kehr, Susanne C.
%A Maia, Francisco C. B.
%D 2023
%J Nano Lett.
%K a
%N 9
%P 3913–3920
%R 0.1021/acs.nanolett.3c00578
%T Graphene nano-optics in the terahertz gap
%U https://doi.org/10.1021/acs.nanolett.3c00578
%V 23
%X Graphene nano-optics at terahertz (THz) frequencies (ν) is theoretically anticipated to feature extraordinary effects. However, interrogating such phenomena is nontrivial, since the atomically thin graphene dimensionally mismatches the THz radiation wavelength reaching hundreds of micrometers. Greater challenges happen in the THz gap (0.1–10 THz) wherein light sources are scarce. To surpass these barriers, we use a nanoscope illuminated by a highly brilliant and tunable free-electron laser to image the graphene nano-optical response from 1.5 to 6.0 THz. For ν < 2 THz, we observe a metal-like behavior of graphene, which screens optical fields akin to noble metals, since this excitation range approaches its charge relaxation frequency. At 3.8 THz, plasmonic resonances cause a field-enhancement effect (FEE) that improves the graphene imaging power. Moreover, we show that the metallic behavior and the FEE are tunable upon electrical doping, thus providing further control of these graphene nano-optical properties in the THz gap.
@article{noauthororeditor,
abstract = {Graphene nano-optics at terahertz (THz) frequencies (ν) is theoretically anticipated to feature extraordinary effects. However, interrogating such phenomena is nontrivial, since the atomically thin graphene dimensionally mismatches the THz radiation wavelength reaching hundreds of micrometers. Greater challenges happen in the THz gap (0.1–10 THz) wherein light sources are scarce. To surpass these barriers, we use a nanoscope illuminated by a highly brilliant and tunable free-electron laser to image the graphene nano-optical response from 1.5 to 6.0 THz. For ν < 2 THz, we observe a metal-like behavior of graphene, which screens optical fields akin to noble metals, since this excitation range approaches its charge relaxation frequency. At 3.8 THz, plasmonic resonances cause a field-enhancement effect (FEE) that improves the graphene imaging power. Moreover, we show that the metallic behavior and the FEE are tunable upon electrical doping, thus providing further control of these graphene nano-optical properties in the THz gap.},
added-at = {2023-10-17T09:51:10.000+0200},
author = {Feres, Flávio H. and Barcelos, Ingrid D. and Cadore, Alisson R. and Wehmeier, Lukas and Nörenberg, Tobias and Mayer, Rafael A. and Freitas, Raul O. and Eng, Lukas M. and Kehr, Susanne C. and Maia, Francisco C. B.},
biburl = {https://www.bibsonomy.org/bibtex/2e5c00a15a95f468fe65a8b1059a07bfb/ctqmat},
day = 01,
description = {Graphene Nano-Optics in the Terahertz Gap | Nano Letters},
doi = {0.1021/acs.nanolett.3c00578},
interhash = {bb22f6b11aec1881bd32c762204ec4d8},
intrahash = {e5c00a15a95f468fe65a8b1059a07bfb},
journal = {Nano Lett.},
keywords = {a},
month = {05},
number = 9,
pages = {3913–3920},
timestamp = {2023-10-17T09:51:10.000+0200},
title = {Graphene nano-optics in the terahertz gap},
url = {https://doi.org/10.1021/acs.nanolett.3c00578},
volume = 23,
year = 2023
}