%0 Journal Article %1 Kinnison2007 %A Kinnison, D. E. %A Brasseur, G. P. %A Walters, S. %A Garcia, R. R. %A Marsh, D. R. %A Sassi, F. %A Harvey, V. L. %A Randall, C. E. %A Emmons, L. %A Lamarque, J. F. %A Hess, P. %A Orlando, J. J. %A Tie, X. X. %A Randel, W. %A Pan, L. L. %A Gettelman, A. %A Granier, C. %A Diehl, T. %A Niemeier, U. %A Simmons, A. J. %D 2007 %I Amer Geophysical Union %J Journal of Geophysical Research-Atmospheres %K STRATOSPHERE-TROPOSPHEREEXCHANGE;GENERAL-CIRCULATIONMODEL;MIDDLEATMOSPHERE;WATER-VAPOR;3-DIMENSIONALSIMULATION;INITIATIVEASSESSMENT;GLOBALSIMULATION;CLIMATEMODEL;MEANAGES;OZONE %N D20 %P D20302 %R 10.1029/2006JD007879 %T Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model %V 112 %X The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long- lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCM1b), (2) the European Centre for Medium- Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO2 and SF6 data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCM1b and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi- biennial oscillation circulation on long- lived tracers and ozone is examined.

@article{Kinnison2007, abstract = {The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long- lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCM1b), (2) the European Centre for Medium- Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO2 and SF6 data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCM1b and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi- biennial oscillation circulation on long- lived tracers and ozone is examined.}, added-at = {2009-06-08T21:16:11.000+0200}, af = {Kinnison, D. E.EOLEOLBrasseur, G. P.EOLEOLWalters, S.EOLEOLGarcia, R. R.EOLEOLMarsh, D. R.EOLEOLSassi, F.EOLEOLHarvey, V. L.EOLEOLRandall, C. E.EOLEOLEmmons, L.EOLEOLLamarque, J. F.EOLEOLHess, P.EOLEOLOrlando, J. J.EOLEOLTie, X. X.EOLEOLRandel, W.EOLEOLPan, L. L.EOLEOLGettelman, A.EOLEOLGranier, C.EOLEOLDiehl, T.EOLEOLNiemeier, U.EOLEOLSimmons, A. J.}, author = {Kinnison, D. E. and Brasseur, G. P. and Walters, S. and Garcia, R. R. and Marsh, D. R. and Sassi, F. and Harvey, V. L. and Randall, C. E. and Emmons, L. and Lamarque, J. F. and Hess, P. and Orlando, J. J. and Tie, X. X. and Randel, W. and Pan, L. L. and Gettelman, A. and Granier, C. and Diehl, T. and Niemeier, U. and Simmons, A. J.}, biburl = {https://www.bibsonomy.org/bibtex/25605ddbdcb119ef74b0bb6760ac8bafc/claas}, c1 = {Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80301 USA.EOLEOLUniv Colorado, Atmospher & Space Phys Lab, Boulder, CO 80309 USA.EOLEOLNOAA, Aeron Lab, Boulder, CO 80305 USA.EOLEOLUniv Paris 06, Serv Aeron, Paris, France.EOLEOLUniv Maryland Baltimore Cty, Goddard Earth Sci & Technol Ctr, Baltimore, MD 21228 USA.EOLEOLMax Planck Inst Meteorol, D-20146 Hamburg, Germany.EOLEOLEuropean Ctr Medium Range Weather Forecasts, Reading RG2 9AX, Berks, England.}, citedreferences = {*WORLD MET ORG, 2003, 47 WORLD MET ORG ; ANDREWS AE, 2001, J GEOPHYS RES-ATMOS, V106, P32295 ; BEY I, 2001, J GEOPHYS RES-ATMOS, V106, P23073 ; BOERING KA, 1996, SCIENCE, V274, P1340 ; BRASSEUR GP, 1997, J GEOPHYS RES-ATMOS, V102, P8909 ; BRASSEUR GP, 1998, J GEOPHYS RES-ATMOS, V103, P28265 ; BRASSEUR GP, 2005, AERONOMY MIDDLE ATMO ; CHIPPERFIELD MP, 1993, J GEOPHYS RES-ATMOSP, V98, P7199 ; CONSIDINE DB, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D15301 ; CRUTZEN PJ, 1991, TELLUS A, V43, P136 ; DOUGLASS AR, 1997, J GEOPHYS RES-ATMOS, V102, P19217 ; DOUGLASS AR, 1999, J GEOPHYS RES-ATMOS, V104, P27545 ; DOUGLASS AR, 2003, J GEOPHYS RES-ATMOS, V108, P94259, ARTN 4259 ; DOUGLASS AR, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D16302 ; ELKINS JW, 1996, GEOPHYS RES LETT, V23, P347 ; EMMONS LK, 2003, J GEOPHYS RES-ATMOS, V108, ARTN 8372 ; EYRING V, 2006, J GEOPHYS RES-ATMOS, V111, ARTN D22308 ; FORKMAN P, 2003, GEOPHYS RES LETT, V30, ARTN 1532 ; GARCIA RR, 2007, J GEOPHYS RES-ATMOS, V112, ARTN D09301 ; GETTELMAN A, 2000, J ATMOS SCI, V57, P3 ; GETTELMAN A, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D22101 ; HALL TM, 1994, J GEOPHYS RES-ATMOSP, V99, P1059 ; HALL TM, 1999, J GEOPHYS RES-ATMOS, V104, P18815 ; HAPPELL JD, 2003, GEOPHYS RES LETT, V30, ARTN 1088 ; HAUGLUSTAINE DA, 1998, J GEOPHYS RES-ATMOS, V103, P28291 ; HAYNES PH, 1991, J ATMOS SCI, V48, P651 ; HOLTON JR, 1995, REV GEOPHYS, V33, P403 ; HOROWITZ LW, 2003, J GEOPHYS RES-ATMOS, V108, ARTN 4784 ; HOUGHTON JT, 2001, CLIMATE CHANGE 2001 ; KULAWIK SS, 2006, IEEE T GEOSCI REMOTE, V44, P1324, DOI ; 10.1109/TGRS.2006.871207 ; LAMARQUE JF, 2006, PALEOCEANOGRAPHY, V21, ARTN PA3006 ; LAWRENCE MG, 1999, J GEOPHYS RES-ATMOS, V104, P26245 ; LEFEVRE F, 1994, J GEOPHYS RES, V99, P8183 ; LEVY H, 1985, J GEOPHYS RES-ATMOSP, V90, P3753 ; LIN SJ, 1996, MON WEATHER REV, V124, P2046 ; LUCKE RL, 1999, J GEOPHYS RES-ATMOS, V104, P18785 ; LUMPE J, 2006, J GEOPHYS RES-ATMOS, V111, ARTN D11301 ; LUMPE JD, 2002, J GEOPHYS RES-ATMOS, V107, ARTN 4575 ; MAHOWALD NM, 2002, J GEOPHYS RES-ATMOS, V107, ARTN 4254 ; MARSH D, 2003, J GEOPHYS RES-ATMOS, V108, ARTN 4109 ; MARSH DR, 2007, IN PRESS J GEOPHYS R ; MCLINDEN CA, 2000, J GEOPHYS RES-ATMOS, V105, P14653 ; MCPETERS RD, 1998, NASATP1998206895 ; MONGESANZ BM, 2007, GEOPHYS RES LETT, V34, ARTN L04801 ; MULLER JF, 1995, J GEOPHYS RES-ATMOS, V100, P16445 ; PAN LL, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D23103 ; PAN LL, 2007, J GEOPHYS RES-ATMOS, V112, ARTN D09316 ; PARK JH, 1999, NASATM1999209554 ; PARK M, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D03302 ; PENNER JE, 1991, J GEOPHYS RES, V96, P959 ; RANDALL CE, 2003, J GEOPHYS RES-ATMOS, V108, ARTN 4367 ; RANDEL WJ, 1998, J ATMOS SCI, V55, P163 ; RANDEL WJ, 2004, J ATMOS SCI, V61, P2133 ; RASCH PJ, 1994, J GEOPHYS RES-ATMOSP, V99, P999 ; RASCH PJ, 1997, J GEOPHYS RES-ATMOS, V102, P28127 ; RAY EA, 1999, J GEOPHYS RES-ATMOS, V104, P26565 ; ROELOFS GJ, 1995, J GEOPHYS RES-ATMOSP, V100, P20983 ; ROSE K, 1989, J GEOPHYS RES-ATMOSP, V94, P16387 ; ROTMAN DA, 2001, J GEOPHYS RES-ATMOS, V106, P1669 ; ROTMAN DA, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D04303 ; SABUTIS JL, 2000, GEOPHYS RES LETT, V27, P3205 ; SASSI F, 2004, J GEOPHYS RES-ATMOS, V109, ARTN D17108 ; SASSI F, 2005, GEOPHYS RES LETT, V32, ARTN L07811 ; SCHMIDT H, 2006, J CLIMATE, V19, P3903 ; SCHOEBERL MR, 2003, J GEOPHYS RES-ATMOS, V108, ARTN 4113 ; SOLOMON S, 1985, J GEOPHYS RES-ATMOS, V90, P2981 ; THOMASON LW, 1997, J GEOPHYS RES-ATMOS, V102, P8967 ; TIAN WS, 2006, J GEOPHYS RES-ATMOS, V111, ARTN D20301 ; TILMES S, 2007, IN PRESS J GEOPHYS R ; UPPALA SM, 2005, Q J ROY METEOR SOC B, V131, P2961, DOI ; 10.1256/qj.04.176 ; VANNOIJE TPC, 2004, J GEOPHYS RES, V109, DOI 10.1029/2004JD004586 ; VOLK CM, 1997, J GEOPHYS RES-ATMOS, V102, P25543 ; WANG YH, 1998, J GEOPHYS RES-ATMOS, V103, P10713 ; WAUGH DW, 2002, REV GEOPHYS, V40, ARTN 1010 ; WILLIAMSON DL, 1994, MON WEATHER REV, V122, P1594 ; WILLIAMSON DL, 1997, NUMERICAL METHODS AT, P279 ; YVONLEWIS SA, 1997, GEOPHYS RES LETT, V24, P1227}, di = {ARTN D20302}, doi = {10.1029/2006JD007879}, file = {Kinnison2007.pdf:Kinnison2007.pdf:PDF}, ga = {224LV}, interhash = {6961103b35ed014b7fb2ecfb9403d9b4}, intrahash = {5605ddbdcb119ef74b0bb6760ac8bafc}, j9 = {J GEOPHYS RES-ATMOS}, ji = {J. Geophys. Res.-Atmos.}, journal = {Journal of Geophysical Research-Atmospheres}, keywords = {STRATOSPHERE-TROPOSPHEREEXCHANGE;GENERAL-CIRCULATIONMODEL;MIDDLEATMOSPHERE;WATER-VAPOR;3-DIMENSIONALSIMULATION;INITIATIVEASSESSMENT;GLOBALSIMULATION;CLIMATEMODEL;MEANAGES;OZONE}, la = {English}, month = {#oct#}, nr = {77}, number = {D20}, pa = {2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA}, pages = {D20302}, pg = {24}, pi = {WASHINGTON}, publisher = {Amer Geophysical Union}, rp = {Kinnison, DE, Natl Ctr Atmospher Res, Div Atmospher Chem, 3450 MitchellEOLEOLLane, Boulder, CO 80301 USA.}, sc = {Meteorology & Atmospheric Sciences}, sn = {0148-0227}, tc = {10}, timestamp = {2009-06-08T21:16:11.000+0200}, title = {Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model}, ut = {ISI:000250449400001}, volume = 112, year = 2007 }